Chitosan-clinoptilolite composite was prepared and tested for removing radiocobalt from aqueous solution. The composite was characterized with Fourier transform infrared spectroscopy, X-ray diffraction analysis and scanning electron microscopy coupled with energy dispersive X-ray analysis. The sorption of Co(II) on chitosanclinoptilolite composite was pH-dependent and ionic strength-independent. The kinetic sorption was fitted well by a pseudo-second-order rate equation. The thermodynamic parameters (DH 0 , DS 0 , DG 0 ) revealed that the sorption of Co(II) on chitosan-clinoptilolite composite was spontaneous and endothermic. The study showed that chitosan-clinoptilolite composite had excellent potential for the treatment of wastewater containing radiocobalt.