volume 160, issue 1, P149-154 2013
DOI: 10.1016/j.combustflame.2012.09.004
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Abstract: a b s t r a c tA two-dimensional model of a weakly buoyant flow over a horizontal wire with surface reaction was developed, using a literature mechanism, to simulate the heat release rate of the catalytic oxidation of methane (2 vol.% in air) over a Pd wire with a porous 1-2 lm PdO surface layer, acquired by wire microcalorimetry over the temperature range of 600-770 K. The experimental and simulation results demonstrate that the catalytic oxidation is characterized by a low-temperature, reaction-controlled r…

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