volume 6, issue 62, P57174-57182 2016
DOI: 10.1039/c6ra08320j
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Abstract: 5For the selective hydrogenation of acetylene to ethylene, the selectivity of Pd catalyst is crucial. However, palladium is present as skin distributed on the surface of Al 2 O 3 support. Pd active sites dispersed on the skin exhibited high activity for acetylene removal, which also inhibited over-hydrogenation of ethylene to ethane and formation of oligomeric species on the catalyst. Therefore, it is significant to accurately control the distribution range of Pd active sites on the support by a feasible rout…

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