volume 156, issue 3, P697-705 2009
DOI: 10.1016/j.combustflame.2008.10.022
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Q. Zhang, M.J. Thomson, H. Guo, F. Liu, G.J. Smallwood

Abstract: Soot aggregate formation in a two-dimensional laminar coflow ethylene/air diffusion flame is studied with a pyrene-based soot model, a detailed sectional aerosol dynamics model, and a detailed radiation model. The chemical kinetic mechanism describes polycyclic aromatic hydrocarbon formation up to pyrene, the dimerization of which is assumed to lead to soot nucleation. The growth and oxidation of soot particles are characterized by the HACA surface mechanism and pyrene-soot surface condensation. The mass rang…

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