“…photocatalysis, [9] surface-enhanced spectroscopy, [10,11] nanolasers, [12] solar cells, [13] and plasmonic circuits. [14] Nanogap devices promise to revolutionize numerous aspects of modern science and technology, but they are currently being held back by the absence of fast, controlled, reliable (high yield), and low-cost methods of fabricating in-plane MNGs with electrode spacings below 10 nm. Typical fabrication methods entail the use of e-beam lithography (EBL), [15][16][17] mechanical break junctions, [5,18,19] electrochemical migration, [20,21] wet chemical methods, [22] atomic layer deposition, [23,24] or focused-ion beam (FIB) milling [25,26] to create the nanogaps (see Table S1, Supporting Information for a comparison of common nanogap fabrication techniques).…”