2020
DOI: 10.1039/c9py01531k
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Abstract: Self-healable, recyclable, and robust polyurethane elastomeric composites by thermally driven Diels–Alder chemistry using inorganic–organic hybrid material as crosslinker.

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Cited by 25 publications
(5 citation statements)
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“…13 In addition, the soft segments can provide chain mobility, which contributes to attachment of the damaged surfaces, and diffusion and entanglement of the molecular chains, 14,15 so polyurethane is widely used for self-healing materials. [16][17][18] Polyurethane can heal through noncovalent bonds such as hydrogen bonding, 19,20 metal-ligand, 21,22 host-guest, 23 π-π stacking 24 ; van der Waals interaction, 25 and interdiffusion, 26 also heal through dynamic covalent bonds such as Diels-Alder reaction, 27,28 disulfide, 29,30 diselenide, 31 ditelluride, 32 imine, 33 hindered urea, 34 or oxime-carbamate. 35 However, the relationship among transparency, self-healing, and structure of polymers needs to be further explored.…”
Section: Introductionmentioning
confidence: 99%
“…13 In addition, the soft segments can provide chain mobility, which contributes to attachment of the damaged surfaces, and diffusion and entanglement of the molecular chains, 14,15 so polyurethane is widely used for self-healing materials. [16][17][18] Polyurethane can heal through noncovalent bonds such as hydrogen bonding, 19,20 metal-ligand, 21,22 host-guest, 23 π-π stacking 24 ; van der Waals interaction, 25 and interdiffusion, 26 also heal through dynamic covalent bonds such as Diels-Alder reaction, 27,28 disulfide, 29,30 diselenide, 31 ditelluride, 32 imine, 33 hindered urea, 34 or oxime-carbamate. 35 However, the relationship among transparency, self-healing, and structure of polymers needs to be further explored.…”
Section: Introductionmentioning
confidence: 99%
“…4h). 25,[45][46][47][48][49][50][51][52][53][54] The poly(TA)/Al composite elastomers can rapidly repair damage and self-heal and is thus a promising candidate for operation in harsh environments.…”
Section: Self-healing and Reprocessing Properties Of Poly(ta)/al Comp...mentioning
confidence: 99%
“…Maleimide‐functionalized graphene oxide sheets and their loading were investigated for the mechanical properties and healing efficiency of the PU composites. [ 142 ] Reports also describe the synthesis and incorporation of maleimide functionalized polyhedral oligomeric silsesquioxane (POSS maleimide isobutyl) [ 56 ] and furfuryl‐modified silica particles [ 143 ] into the design of dynamic DA‐crosslinked PU networks.…”
Section: Fabrication Of Self‐healable Heterogeneous Pu Compositesmentioning
confidence: 99%