2019
DOI: 10.1021/acs.nanolett.9b02835
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Abstract: Silicon-core–carbon-shell nanoparticles have been widely studied as promising candidates for the replacement of graphite in commercial lithium-ion batteries. Over more than 10 years of R&D, the many groups actively working in this field have proposed a profusion of distinctive nanomaterial designs. This broad variety makes it extremely challenging to establish mechanistic insight into how fundamental material structure and properties affect battery performance. In particular, the interplay between the characte… Show more

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Cited by 76 publications
(53 citation statements)
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“…In addition to graphitic carbon materials, amorphous carbon has also been extensively studied for LIBs [64][65][66]. Amorphous carbon, categorized into hard carbon and soft carbon, has many excellent characteristics, including poor crystallinity, large lattice spacing, and high compatibility with the electrolyte.…”
Section: Carbonaceous Materialsmentioning
confidence: 99%
“…In addition to graphitic carbon materials, amorphous carbon has also been extensively studied for LIBs [64][65][66]. Amorphous carbon, categorized into hard carbon and soft carbon, has many excellent characteristics, including poor crystallinity, large lattice spacing, and high compatibility with the electrolyte.…”
Section: Carbonaceous Materialsmentioning
confidence: 99%
“…Various methods have been developed to settle these problems, such as reducing the size of Si particles to nanoscale, [12–14] building the coating layer, [15,16] doping hetero‐element, [17–19] designing porous structure, [20–22] and introducing inert components [23–26] . Simultaneously, carbon materials received extensive research as coating layer for Si anode materials due to its high conductivity, superior structural stability (negligible volume expansion), and stable SEI layers.…”
Section: Introductionmentioning
confidence: 99%
“…In response to these bottlenecks, the fabrication of silicon/carbon composites has been highlighted as a promising strategy to overcome the rapid capacity decay of silicon anode . The carbon encapsulation layer not only increases the electronic conductivity of the entire electrode, but also stabilizing the silicon core during rapid cycling .…”
Section: Introductionmentioning
confidence: 99%