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A graphene coated microfiber Bragg grating (GMFBG) for gas sensing is reported in this Letter. Taking advantage of the surface field enhancement and gas absorption of a GMFBG, we demonstrate an ultrasensitive approach to detect the concentration of chemical gas. The obtained sensitivities are 0.2 and 0.5 ppm for NH3 and xylene gas, respectively, which are tens of times higher than that of a GMFBG without graphene for tiny gas concentration change detection. Experimental results indicate that the GMFBG-based NH3 gas sensor has fast response due to its highly compact structure. Such a miniature fiber-optic element may find applications in high sensitivity gas sensing and trace analysis.

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Chemical sensing is one of the most important applications of nanoscience, whose ultimate aim is to seek higher sensitivity. In recent years, graphene with intriguing quantum properties has spurred dramatic advances ranging from materials science to optoelectronics and mechanics, showing its potential to realize individual molecule solid-state sensors. However, for optical sensing the single atom thickness of graphene greatly limits the light-graphene interactions, bottlenecking their performances. Here we demonstrate a novel approach based on the forward phase-matched Brillouin optomechanics in a graphene inner-deposited high Q (>2 × 10) microfluidic resonator, expanding the "electron-photon" interaction in conventional graphene optical devices to the "electron-phonon-photon" process. The molecular adsorption induced surface elastic modulation in graphene enables the Brillouin optomechanical modes (mechanical Q ≈ 43,670) extremely sensitive (200 kHz/ppm) in ammonia gas detection, achieving a noise equivalent detection limit down to 1 ppb and an unprecedented dynamic range over five orders-of-magnitude with fast response. This work provides a new platform for the researches of graphene-based optomechanics, nanophotonics, and optical sensing.