Lithium niobate (LN), an outstanding and versatile material, has influenced our daily life for decades: from enabling high-speed optical communications that form the backbone of the Internet to realizing radio-frequency filtering used in our cell phones. This half-century-old material is currently embracing a revolution in thin-film LN integrated photonics. The success of manufacturing wafer-scale, high-quality, thin films of LN on insulator (LNOI), accompanied with breakthroughs in nanofabrication techniques, have made high-performance integrated nanophotonic components possible. With rapid development in the past few years, some of these thin-film LN devices, such as optical modulators and nonlinear wavelength converters, have already outperformed their legacy counterparts realized in bulk LN crystals. Furthermore, the nanophotonic integration enabled ultra-low-loss resonators in LN, which unlocked many novel applications such as optical frequency combs and quantum transducers. In this Review, we cover-from basic principles to the state of the art-the diverse aspects of integrated thinfilm LN photonics, including the materials, basic passive components, and various active devices based on electro-optics, all-optical nonlinearities, and acousto-optics. We also identify challenges that this platform is currently facing and point out future opportunities. The field of integrated LNOI photonics is advancing rapidly and poised to make critical impacts on a broad range of applications in communication, signal processing, and quantum information.

Physical systems with discrete energy levels are ubiquitous in nature and are fundamental building blocks of quantum technology. Realizing controllable artificial atom-and molecule-like systems for light would allow for coherent and dynamic control of the frequency, amplitude and phase of photons. In this work, we demonstrate a photonic molecule with two distinct energy-levels and control it by external microwave excitation. We show signature two-level dynamics including microwave induced photonic Autler-Townes splitting, Stark shift, Rabi oscillation and Ramsey interference. Leveraging the coherent control of optical energy, we show on-demand photon storage and retrieval in optical microresonators by reconfiguring the photonic molecule into a bright-dark mode pair. These results of dynamic control of light in a programmable and scalable electro-optic platform open doors to applications in microwave photonic signal processing, quantum photonics in the frequency domain, optical computing concepts and simulations of complex physical systems.

Crystals are ubiquitous in nature and are at the heart of material research, solid-state science, and quantum physics. Unfortunately, the controllability of solid-state crystals is limited by the complexity of many-body dynamics and the presence of defects. In contrast, synthetic crystal structures, realized by, e.g.,  optical lattices, have recently enabled the investigation of various physical processes in a controllable manner, and even the study of new phenomena. Past realizations of synthetic optical crystals were, however, limited in size and dimensionality. Here we theoretically propose and experimentally demonstrate optical frequency crystal of arbitrary dimensions, formed by hundreds of coupled spectral modes within an on-chip electro-optic frequency comb. We show a direct link between the measured optical transmission spectrum and the density of states of frequency crystals in one, two, three, and four dimensions, with no restrictions to further expanding the dimensionality. We demonstrate that the generation of classical electro-optic frequency comb can be modeled as a process described by random walks in a tight-binding model, and we have verified this by measuring the coherent distribution of optical steady states. We believe that our platform is a promising candidate for exploration of topological and quantum photonics in the frequency domain.

Linking superconducting quantum devices to optical fibers via microwave-optical quantum transducers may enable large-scale quantum networks. For this application, transducers based on the Pockels electro-optic (EO) effect are promising for their direct conversion mechanism, high bandwidth, and potential for low-noise operation. However, previously demonstrated EO transducers require large optical pump power to overcome weak EO coupling and reach high efficiency. Here, we create an EO transducer in thin-film lithium niobate, a platform that provides low optical loss and strong EO coupling. We demonstrate on-chip transduction efficiencies of up to and of optical pump power. The transduction efficiency can be improved by further reducing the microwave resonator’s piezoelectric coupling to acoustic modes, increasing the optical resonator quality factor to previously demonstrated levels, and changing the electrode geometry for enhanced EO coupling. We expect that with further development, EO transducers in thin-film lithium niobate can achieve near-unity efficiency with low optical pump power.