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▪ Abstract  Yttrium aluminum garnet (YAG) (Y3Al5O12) single crystals doped with active species such as Nd and Yb have been used as laser media in solid-state lasers requiring high energy and excellent beam quality. This is because single crystals have extremely high thermal mechanical properties and optical qualities and because they enable high-efficiency laser oscillation. In 1995 the authors, using polycrystalline Nd:YAG, demonstrated a high-efficiency laser that was comparable to a single-crystal laser. Subsequently, single-longitudinal-mode oscillation, green and blue laser oscillation, and ultrashort-pulse laser oscillation were reported. Using the ceramic powder approach, the authors developed a composite laser element with a complicated structure that could not be produced by crystal growth techniques. This review discusses problems of conventional single-crystal growth, the fabrication and characteristics of ceramic lasers, laser oscillation properties (continuous-wave and pulse operation), light-scattering sources in ceramics, and typical applications of ceramic lasers.

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This paper reports recent progress in the production of polycrystalline Nd:YAG (Y 3 Al 5 O 12 ), Nd:YSAG (Y 3 Sc 1.0 Al 4.0 O 12 ), Yb:YSAG ceramics, and a Nd-doped YAG single crystal with an almost perfect pore-free structure by advanced ceramic processing. The laser conversion efficiency of pore-free polycrystalline Nd-and Yb-doped ceramics is extremely high, and their optical qualities are comparable with that of commercial high-quality Nd:YAG single crystals. We have also succeeded in the fabrication of a Nd:YAG single crystal, which can be used for laser oscillation, by the solid-state reaction method. Laser oscillation efficiency was very low when the pores remained inside the single crystal; however, the laser oscillation efficiency of the pore-free Nd:YAG single crystal was slightly higher than that of polycrystalline Nd:YAG ceramics having high optical quality. From this fact, it was recognized that optical scattering occurs mainly in the residual pores inside the Nd:YAG ceramics and the scattering at the grain boundary is very less. In addition, we confirmed that a heavily doped Nd:YAG single crystal can be fabricated by the sintering method. Moreover, we have demonstrated the fabrication of a composite ceramic with complicated structures without the need for precise polishing and diffusion bonding. Advanced ceramic processing, which enables design flexibility of the laser element, presented in this work is important in the development of a high-performance laser (high efficiency, high beam quality, and high output energy, etc.) I. IntroductionJ ournal

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