The Gravity Recovery and Climate Experiment (GRACE) data have been extensively used to evaluate the total terrestrial water storage anomalies (TWSA) from hydrological models. However, which individual water storage components (i.e., soil moisture storage anomalies (SMSA) or groundwater water storage anomalies (GWSA)) cause the discrepancies in TWSA between GRACE and hydrological models have not been thoroughly investigated or quantified. In this study, we applied GRACE mass concentration block (mascon) solutions to evaluate the spatio-temporal TWSA trends (2003–2014) from seven prevailing hydrological models (i.e., Noah-3.6, Catchment Land Surface Model (CLSM-F2.5), Variable Infiltration Capacity macroscale model (VIC-4.1.2), Water—Global Assessment and Prognosis (WaterGAP-2.2d), PCRaster Global Water Balance (PCR-GLOBWB-2), Community Land Model (CLM-4.5), and Australian Water Resources Assessment Landscape model (AWRA-L v6)) in Australia and, more importantly, identified which individual water storage components lead to the differences in TWSA trends between GRACE and hydrological models. The results showed that all of the hydrological models employed in this study, except for CLM-4.5 model, underestimated the GRACE-derived TWSA trends. These underestimations can be divided into three categories: (1) ignoring GWSA, e.g., Noah-3.6 and VIC-4.1.2 models; (2) underrating both SMSA and GWSA, e.g., CLSM-F2.5, WaterGAP-2.2d, and PCR-GLOBWB-2 models; (3) deficiently modeling GWSA, e.g., AWRA-L v6 model. In comparison, CLM-4.5 model yielded the best agreement with GRACE but overstated the GRACE-derived TWSA trends due to the overestimation of GWSA. Our results underscore that GRACE mascon solutions can be used as a valuable and efficient validation dataset to evaluate the spatio-temporal performance of hydrological models. Confirming which individual water storage components result in the discrepancies in TWSA between GRACE and hydrological models can better assist in further hydrological model development.
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