Neutron diffraction and calorimetric measurements are used to study the
field-induced quantum phase transition in
piperazinium-Cu$_2$(Cl$_{1-x}$Br$_x$)$_6$ ($x=0$, x=3.5% and x=7.5%), a
prototypical quantum antiferromagnet with random bonds. The critical indexes
$\phi$ and $\beta$ are determined. The findings contradict some original
predictions for Bose Glass based on the assumption $z=d$, but are consistent
with recent theoretical results implying $z
Inelastic neutron scattering is used to measure spin excitations in fully deuterated single crystal samples of the strong-leg antiferromagnetic S = 1/2 spin ladder compound (C7D10N)2CuBr4. Sharp resolution-limited magnons are observed across the entire one-dimensional Brillouin zone. The results validate the previously proposed symmetric spin ladder model and provide a reliable estimate of the relevant exchange interactions. arXiv:1105.4832v1 [cond-mat.str-el]
We review a strategy for targeted synthesis of large single crystal samples of prototype quantum magnets for inelastic neutron scattering experiments. Four case studies of organic copper halogenide S = 1/2 systems are presented. They are meant to illustrate that exciting experimental results pertaining to forefront many-body quantum physics can be obtained on samples grown using very simple techniques, standard laboratory equipment, and almost no experience in in advanced crystal growth techniques.
The effect of disorder is studied on the field-induced quantum phase transition in the frustrated spin-ladder compound H8C4SO2·Cu2(Cl1−xBrx)4 using bulk magnetic and thermodynamic measurements. The parent material (x = 0) is a quantum spin liquid, which in applied fields is known to form a magnon condensate with long-range helimagnetic order. We show that bond randomness introduced by a chemical substitution on the non-magnetic halogene site destroys this phase transition at very low concentrations, already for x = 0.01. The extreme fragility of the magnon condensate is attributed to random frustration in the incommensurate state.
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