Optical soliton molecules exhibiting behaviors analogous to matter molecules have been the hotspot in the dissipative system for decades. Based on the dispersion Fourier transformation technique, the real-time spectral interferometry has become the popular method to reveal the internal dynamics of soliton molecules. The rising degrees of freedom in pace with the increased constitutes of soliton molecules yield more intriguing sights into the internal motions. Yet the soliton molecules with three or more pulses are rarely investigated owing to the exponentially growing complexity. Here, we present both experimental and theoretical studies on the soliton molecules containing three solitons. Different assemblies of the constitutes are categorized as different types of soliton triplet akin to the geometric isomer, including equally-spaced triplet and unequally-spaced triplet. Typical soliton triplets with different dynamics including regular internal motions, hybrid phase dynamics and complex dynamics involving separation evolution are experimentally analyzed and theoretically simulated. Specifically, the energy difference which remains elusive in experiments are uncovered through the simulation of diverse triplets with plentiful dynamics. Moreover, the multi-dimensional interaction space is proposed to visualize the internal motions in connection with the energy exchange, which play significant roles in the interplays among the solitons. Both the experimental and numerical simulations on the isomeric soliton triplets would release a larger number of degrees of freedom and motivate the potentially artificial configuration of soliton molecules for various ultrafast applications, such as all-optical buffering and multiple encoding for telecommunications.
Self-assembly of particle-like dissipative solitons, in the presence of mutual interactions, emphasizes the vibrant concept of soliton molecules in varieties of laser resonators. Controllable manipulation of the molecular patterns, held by the degrees of freedom of internal motions, still remains challenging to explore more efficient and subtle tailoring approaches for the increasing demands. Here, we report a new phase-tailored quaternary encoding format based on the controllable internal assembly of dissipative soliton molecules. Artificial manipulation of the energy exchange of soliton-molecular elements stimulates the deterministic harnessing of the assemblies of internal dynamics. Self-assembled soliton molecules are tailored into four phase-defined regimes, thus constituting the phase-tailored quaternary encoding format. Such phase-tailored streams are endowed with great robustness and are resistant to significant timing jitter. All these results experimentally demonstrate the programmable phase tailoring and exemplify the application of the phase-tailored quaternary encoding, prospectively promoting high-capacity all-optical storage.
Self-assembly of optical solitons propagating in nonlinear dissipative systems spreads the concept of soliton molecules. Assisted with the real-time spectral interferometry, plentiful internal dynamics has been probed within the multi-pulse patterns, emphasizing the striking analogies with the matter molecules. Therefrom, these particle-like behaviors would yield more intriguing landscapes towards the extended degrees of freedom considering increased constituents. Here, we transfer the concept of 'isomer' to the experimental investigation on the unexplored isomeric dynamics of soliton molecules in parallel. Particularly, two isomers for soliton triplets and four isomers for soliton quadruplets are captured under different self-assembled forms, within each of which the binding separations and relative phases of the constituents are governed by mutual soliton interactions. With the diverse separation-phase evolving trajectories mapped in the interaction plane, the detailed insights of the temporal distribution and the transient dynamics are displayed with respect to a panorama of the isomeric dynamics. The perspective of optical isomers shed new light on the analogy with matter molecules, and the underlying isomeric dynamics may stimulate the artificial manipulation of various soliton molecules for ultrafast applications.
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