Small-scale pumps will be the heartbeat of many future micro/ nanoscale platforms. However, the integration of small-scale pumps is presently hampered by limited flow rate with respect to the input power, and their rather complicated fabrication processes. These issues arise as many conventional pumping effects require intricate moving elements. Here, we demonstrate a system that we call the liquid metal enabled pump, for driving a range of liquids without mechanical moving parts, upon the application of modest electric field. This pump incorporates a droplet of liquid metal, which induces liquid flow at high flow rates, yet with exceptionally low power consumption by electrowetting/deelectrowetting at the metal surface. We present theory explaining this pumping mechanism and show that the operation is fundamentally different from other existing pumps. The presented liquid metal enabled pump is both efficient and simple, and thus has the potential to fundamentally advance the field of microfluidics.E ngines are systems that convert different kinds of energy into mechanical motion, which are used in various microscale systems, including laboratory-on-a-chip microreactors (1-3), microelectromechanical (MEMS) actuators (4), and microscale heat exchangers (5, 6), to name just a few. Some of the most important members of the engine family are liquid pumps. In the small-scale regime, such pumps can be mainly classified into mechanical and nonmechanical. For mechanical pumps, the driving force is generated by moving parts that are energized using piezoelectric (7), electrostatic (8), thermopneumatic (9), pneumatic (10), electromagnetic (11) effects, or deformation through electrowetting (12). Mechanical pumping systems have several drawbacks, which largely stem from the fact that moving parts cause energy loses due to heat generated by friction and their rather complicated fabrication processes (13,14). In addition, the existence of moving parts increases the potential for failure, which can become acute in complex systems and which could potentially include numerous pumps. Among the varieties of mechanical pumps, only piezoelectric units can produce high flow rates as large as 20,000 μL/min at relatively low input power (>50 mW) (13, 15). However, piezoelectric units generally require operating voltages larger than 100 V (13, 15). Alternatively, nonmechanical pumps with no moving parts generate a driving force using ions energized via electrohydrodynamic (16), electroosmotic (17), or electrochemical (18, 19) effects. However, ion pumps are generally only applicable for low-conductivity liquids, produce relatively low flow rates, and need very high voltages (in the order of kilovolts) to operate (13). Therefore, a pumping system with no moving parts, high flow rate, and low power consumption is ideal for many present-day and emerging applications in microfluidic systems. An ambitious vision is that such pumps can potentially be used for moving small objects on demand, assembling them to create new structures, or could ...
Liquid metal marbles that are droplets of liquid metal encapsulated by micro‐ or nanoparticles are introduced. Droplets of galinstan liquid metal are coated with insulators (including Teflon and silica) and semiconductors (including WO3, TiO2, MoO3, In2O3 and carbon nanotubes) by rolling over a powder bed and also by submerging in colloidal suspensions. It is shown that these marbles can be split and merged, can be suspended on water, and are even stable when moving under the force of gravity and impacting a flat solid surface. Furthermore, the marble coating can operate as an active electronic junction and the nanomaterial coated liquid metal marble can act as a highly sensitive electrochemical based heavy metal ion sensor. This new element thus represents a significant platform for the advancement of research into soft electronics.
Several gallium-based liquid metal alloys are liquid at room temperature. As 'liquid', such alloys have a low viscosity and a high surface tension while as 'metal', they have high thermal and electrical conductivities, similar to mercury. However, unlike mercury, these liquid metal alloys have low toxicity and a negligible vapor pressure, rendering them much safer. In comparison to mercury, the distinguishing feature of these alloys is the rapid formation of a self-limiting atomically thin layer of gallium oxide over their surface when exposed to oxygen. This oxide layer changes many physical and chemical properties of gallium alloys, including their interfacial and rheological properties, which can be employed and modulated for various applications in microfluidics. Injecting liquid metal into microfluidic structures has been extensively used to pattern and encapsulate highly deformable and reconfigurable electronic devices including electrodes, sensors, antennas, and interconnects. Likewise, the unique features of liquid metals have been employed for fabricating miniaturized microfluidic components including pumps, valves, heaters, and electrodes. In this review, we discuss liquid metal enabled microfluidic components, and highlight their desirable attributes including simple fabrication, facile integration, stretchability, reconfigurability, and low power consumption, with promising applications for highly integrated microfluidic systems.
Conductive elastic composites have been used widely in soft electronics and soft robotics. These composites are typically a mixture of conductive fillers within elastomeric substrates. They can sense strain via changes in resistance resulting from separation of the fillers during elongation. Thus, most elastic composites exhibit a negative piezoconductive effect, i.e. the conductivity decreases under tensile strain. This property is undesirable for stretchable conductors since such composites may become less conductive during deformation. Here, we report a liquid metal-filled magnetorheological elastomer comprising a hybrid of fillers of liquid metal microdroplets and metallic magnetic microparticles. The composite’s resistivity reaches a maximum value in the relaxed state and drops drastically under any deformation, indicating that the composite exhibits an unconventional positive piezoconductive effect. We further investigate the magnetic field-responsive thermal properties of the composite and demonstrate several proof-of-concept applications. This composite has prospective applications in sensors, stretchable conductors, and responsive thermal interfaces.
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