The iron chalcogenide Fe(1+y)(Te(1-x)Se(x)) is structurally the simplest of the Fe-based superconductors. Although the Fermi surface is similar to iron pnictides, the parent compound Fe(1+y)Te exhibits antiferromagnetic order with an in-plane magnetic wave vector (pi,0) (ref. 6). This contrasts the pnictide parent compounds where the magnetic order has an in-plane magnetic wave vector (pi,pi) that connects hole and electron parts of the Fermi surface. Despite these differences, both the pnictide and chalcogenide Fe superconductors exhibit a superconducting spin resonance around (pi,pi) (refs 9, 10, 11). A central question in this burgeoning field is therefore how (pi,pi) superconductivity can emerge from a (pi,0) magnetic instability. Here, we report that the magnetic soft mode evolving from the (pi,0)-type magnetic long-range order is associated with weak charge carrier localization. Bulk superconductivity occurs as magnetic correlations at (pi,0) are suppressed and the mode at (pi, pi) becomes dominant for x>0.29. Our results suggest a common magnetic origin for superconductivity in iron chalcogenide and pnictide superconductors.

We investigate the phase diagram of TmB4, an Ising magnet on a frustrated Shastry-Sutherland lattice, by neutron diffraction and magnetization experiments. At low temperature we find Néel order at low field, ferrimagnetic order at high field, and an intermediate phase with magnetization plateaus at fractional values M/M_(sat)=1/7,1/8,1/9,... and spatial stripe structures. Using an effective S=1/2 model and its equivalent two-dimensional fermion gas we suggest that the magnetic properties of TmB4 are related to the fractional quantum Hall effect of a 2D electron gas.

Effect of pressure on magnetic properties of magnetic nanoparticles, based on Prussian blue analogues, were studied in pressures up to 1.2 GPa. The Mn 3 [Cr(CN) 6 ] 2 · nH 2 O and Ni 3 [Cr(CN) 6 ] 2 · nH 2 O nanoparticles were prepared by reverse micelle technique. Transmission electron microscopy images show nanoparticles with average diameter of about 3.5 nm embedded in an organic matrix. The characteristic X-ray peaks of nanoparticles are more diffused and broader. Systems of nanoparticles behave as systems of interacting magnetic particles. The Curie temperature TC is reduced from T C = 56 K for Ni-Prussian blue analogues to T C = 21 K for Ni-nanoparticles system and from TC = 65 K for Mn-Prussian blue analogues to T C = 38 K for Mn-nanoparticles system. One can explain this reduction of the Curie temperature and of the saturated magnetization µs by dispersion of nanoparticles in an organic matrix i.e. by a dilution effect. Applied pressure leads to a remarkable increase in T C for system of Mn-nanoparticles (∆T C /∆p = +13 K/GPa) and to only slight decrease in T C for system of Ni-nanoparticles (∆T C /∆p = −3 K/GPa). The pressure effect follows behavior of the mother Prussian blue analogues under pressure. The increase in saturated magnetization, attributed to compression of the organic matrix, is very small. PACS numbers: 75.30.Cr, 75.50.Ee, 75.50.Gg, 75.50.Xx (489) 490 A. Zentko et al.

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Magnetic structure of single crystalline TmB 4 has been studied by magnetization, magnetoresistivity, and specific heat measurements. A complex phase diagram with different antiferromagnetic phases was observed below T N1 = 11.7 K. Besides the plateau at half-saturated magnetization (1/2 M S ), also plateaus at 1/9, 1/8 and 1/7 of MS were observed as a function of applied magnetic field B c. From additional neutron scattering experiments on TmB4, we suppose that these plateaus arise from a stripe structure which appears to be coherent domain boundaries between antiferromagnetic-ordered blocks of 7 or 9 lattice constants. The received results suggest that the frustration among the Tm 3+ magnetic ions, which maps to a geometrically frustrated Shastry-Sutherland lattice, leads to a strong competition between antiferromagnetic and ferromagnetic order. Thus, stripe structures in intermediate field appear to be the best way to minimize the magnetostatic energy against other magnetic interactions among the Tm ions combined with very strong Ising anisotropy.PACS numbers: 75.30.Kz, 75.25.+z IntroductionRare earth tetraborides REB 4 crystallize in a tetragonal structure with the space group P 4/mbm, where the RE ions map to a Shastry-Sutherland type geometrically frustrated lattice (SSL) in the c-plane. It was shown that all heavy REB 4 (RE = Tb, Dy, Ho, Er, Tm) exhibit a strong Ising-like anisotropy which orients the RE magnetic moments along the c-axis, and complex phase dia-

Magnetization, specific heat, and neutron scattering measurements were performed to study a magnetic transition in jarosite, a spin-5 2 kagome lattice antiferromagnet. When a magnetic field is applied perpendicular to the kagome plane, magnetizations in the ordered state show a sudden increase at a critical field Hc, indicative of the transition from antiferromagnetic to ferromagnetic states. This sudden increase arises as the spins on alternate kagome planes rotate 180• to ferromagnetically align the canted moments along the field direction. The canted moment on a single kagome plane is a result of the Dzyaloshinskii-Moriya interaction. For H < Hc, the weak ferromagnetic interlayer coupling forces the spins to align in such an arrangement that the canted components on any two adjacent layers are equal and opposite, yielding a zero net magnetic moment. For H > Hc, the Zeeman energy overcomes the interlayer coupling causing the spins on the alternate layers to rotate, aligning the canted moments along the field direction. Neutron scattering measurements provide the first direct evidence of this 180• spin rotation at the transition.