The rate of supernovae (SNe) in our local galactic neighborhood within a distance of ~100 parsec from Earth (1 parsec (pc)=3.26 light years) is estimated at 1 SN every 2-4 million years (Myr), based on the total SN-rate in the Milky Way (2.0±0.7 per century1,2). Recent massive-star and SN activity in Earth’s vicinity may be evidenced by traces of radionuclides with half-lives t1/2 ≤100 Myr3-6, if trapped in interstellar dust grains that penetrate the Solar System (SS). One such radionuclide is 60Fe (t1/2=2.6 Myr)7,8 which is ejected in supernova explosions and winds from massive stars1,2,9. Here we report that the 60Fe signal observed previously in deep-sea crusts10,11, is global, extended in time and of interstellar origin from multiple events. Deep-sea archives from all major oceans were analyzed for 60Fe deposition via accretion of interstellar dust particles. Our results, based on 60Fe atom-counting at state-of-the-art sensitivity8, reveal 60Fe interstellar influxes onto Earth 1.7–3.2 Myr and 6.5–8.7 Myr ago. The measured signal implies that a few percent of fresh 60Fe was captured in dust and deposited on Earth. Our findings indicate multiple supernova and massive-star events during the last ~10 Myr at nearby distances ≤100 pc.

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The Fukushima nuclear accident in March 2011 has released a large amount of radioactive pollutants to the environment. Of the pollutants, iodine-129 is a long-lived radionuclide and will remain in the environment for millions of years. This work first report levels and inorganic speciation of (129)I in seawater depth profiles collected offshore Fukushima in June 2011. Significantly elevated (129)I concentrations in surface water were observed with the highest (129)I/(127)I atomic ratio of 2.2 × 10(-9) in the surface seawater 40 km offshore Fukushima. Iodide was found as the dominant species of (129)I, while stable (127)I was mainly in iodate form, reflecting the fact that the major source of (129)I is the direct liquid discharges from the Fukushima NPP. The amount of (129)I directly discharged from the Fukushima Dai-ichi nuclear power plant to the sea was estimated to be 2.35 GBq, and about 1.09 GBq of (129)I released to the atmosphere from the accident was deposited in the sea offshore Fukushima. A total release of 8.06 GBq (or 1.2 kg) of (129)I from the Fukushima accident was estimated. These Fukushima-derived (129)I data provide necessary information for the investigation of water circulation and geochemical cycle of iodine in the northwestern Pacific Ocean in the future.

Systematic investigations and experience from several application projects on small carbon samples over a number of years have resulted in measuring the radiocarbon content of 10 μg C samples with an overall precision of typically 1%. A substantial reduction of the carbon contamination during graphitization was achieved, resulting in 31±30 ng modern and <100 ng 14C-free carbon. Thus, graphitization is no longer the limiting factor because earlier sample preparation steps usually introduce much larger contamination. The method has been extended to a variety of materials and applied to various projects. Realistic conditions for procedure development can only be achieved in the context of applications on true samples; methods developed are the lyophilization of samples in solution, combustion, ultraviolet oxidation, or carbonate hydrolysis with phosphoric acid, which allows to prepare samples for a wide range of applications. Insights gained from systematic investigations and from real applications are presented.

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