Colloidal nanoplatelets (NPLs), a class of semiconductor nanocrystals, have attracted considerable attention as a promising gain material for their ultralow amplified spontaneous emission (ASE) and lasing thresholds. However, there exist spectral gaps, especially in the green-color range, that NPLs cannot fully cover. The recently developed CdSe/CdSeS core/ alloyed-crown NPLs with excellent tunability across the greencolor range offer the possibility to remedy this deficiency. Here, the ASE and lasing characteristics of this new type of NPL are investigated. A remarkably low ASE threshold of 16 μJ/cm 2 at 522 nm is measured, the lowest among core/crown NPLs. Microlasers are fabricated by spin-coating them on second-order distributed feedback (DFB) cavities developed in silicon nitride (SiN) substrates. The microlasers exhibit an ultralow lasing threshold of 9 μJ/cm 2 at 522 nm. Moreover, they can cover a spectral range of 505−535 nm with all clean single-mode emissions. Picosecond time-and spectral-resolved photoluminescence (PL) spectroscopy reveals that the gain band is determined by the biexciton emission bandwidth. The vigorous development of NPLs with low lasing thresholds in a broad spectral range will greatly facilitate the realization of nanocrystal-based lasers.

Two-dimensional perovskite crystals have attracted significant attention for their diverse optoelectronic characteristics, owing to their superior semiconducting properties. However, the majority of studies to date have focused on single crystals, which pose challenges for integration into device arrays due to their incompatibility with selective growth or conventional lithography techniques. Here, a facile one-step solution process for synthesizing 2D perovskite crystal arrays is proposed through meniscus-guided coating on patterned substrates. We further utilized this method for the synthesis of lateral heterostructure nanoplate arrays. Six different 2D perovskite nanoplate arrays, including epitaxial heterostructures, are successfully realized. Optical and crystallographic characterizations show the high optical performance and crystallinity of the nanoplates. Moreover, this method is further employed to prepare high-performance 2D perovskite nanoplate photosensor arrays. This strategy can be utilized as a guideline for the fundamental investigation of optical properties and the development of high-performance optoelectronics of perovskite materials including photosensors and displays.