The existence of a nematic phase transition in iron-chalcogenide superconductors poses an intriguing question about its impact on superconductivity. To understand the nature of this unique quantum phase transition, it is essential to study how the electronic structure changes across this transition at low temperatures. Here, we investigate the evolution of the Fermi surfaces and electronic interactions across the nematic phase transition of FeSe 1−x S x using Shubnikov-de Haas oscillations in high magnetic fields up to 45 T in the low temperature regime down to 0.4 K. Most of the Fermi surfaces of FeSe 1−x S x monotonically increase in size except for a prominent low frequency oscillation associated with a small, but highly mobile band, which disappears at the nematic phase boundary near x~0.17, indicative of a topological Lifshitz transition. The quasiparticle masses are larger inside the nematic phase, indicative of a strongly correlated state, but they become suppressed outside it. The experimentally observed changes in the Fermi surface topology, together with the varying degree of electronic correlations, will change the balance of electronic interactions in the multi-band system FeSe 1−x S x and promote different k z-dependent superconducting pairing channels inside and outside the nematic phase.

Iron-based chalcogenides are complex superconducting systems in which orbitally-dependent electronic correlations play an important role. Here, using high-resolution angle-resolved photoemission spectroscopy, we investigate the effect of these electronic correlations outside the nematic phase in the tetragonal phase of superconducting FeSe1−xSx (x = 0, 0.18, 1). With increasing sulfur substitution, the Fermi velocities increase significantly and the band renormalizations are suppressed towards a factor of 1.5 − 2 for FeS. Furthermore, the chemical pressure leads to an increase in the size of the quasi-two dimensional Fermi surface, compared with that of FeSe, however, it remains smaller than the predicted one from first principle calculations for FeS. Our results show that the isoelectronic substitution is an effective way to tune electronic correlations in FeSe1−xSx, being weakened for FeS with a lower superconducting transition temperature. This suggests indirectly that electronic correlations could help to promote higher-Tc superconductivity in FeSe.

Understanding superconductivity requires detailed knowledge of the normal electronic state from which it emerges. A nematic electronic state that breaks the rotational symmetry of the lattice can potentially promote unique scattering relevant for superconductivity. Here, we investigate the normal transport of superconducting FeSe1−xSx across a nematic phase transition using high magnetic fields up to 69 T to establish the temperature and field-dependencies. We find that the nematic state is an anomalous non-Fermi liquid, dominated by a linear resistivity at low temperatures that can transform into a Fermi liquid, depending on the composition x and the impurity level. Near the nematic end point, we find an extended temperature regime with ∼ T 1.5 resistivity. The transverse magnetoresistance inside the nematic phase has as a ∼ H 1.55 dependence over a large magnetic field range and it displays an unusual peak at low temperatures inside the nematic phase. Our study reveals anomalous transport inside the nematic phase, driven by the subtle interplay between the changes in the electronic structure of a multi-band system and the unusual scattering processes affected by large magnetic fields and disorder.Magnetic field is a unique tuning parameter that can suppress superconductivity to reveal the normal low-temperature electronic behavior of many unconventional superconductors [1,2]. High-magnetic fields can also induce new phases of matter, probe Fermi surfaces and determine the quasi-particle masses from quantum oscillations in the proximity of quantum critical points [1,3]. In unconventional superconductors, close to antiferromagnetic critical regions, an unusual scaling between a linear resistivity in temperature and magnetic fields was found [4,5]. Magnetic fields can also induce metal-toinsulator transitions, as in hole-doped cuprates, where superconductivity emerges from an exotic electronic ground state [2].FeSe is a unique bulk superconductor with T c ∼ 9 K which displays a variety of complex and competing electronic phases [6]. FeSe is a bad metal at room temperature and it enters a nematic electronic state below T s ∼ 87 K. This nematic phase is characterized by multi-band shifts driven by orbital ordering that lead to Fermi surface distortions [6,7]. Furthermore, the electronic ground state is that of a strongly correlated system and the quasiparticle masses display orbital-dependent enhancements [7,8]. FeSe shows no long-range magnetic order at ambient pressure, but complex magnetic fluctuations are present at high energies over a large temperature range [9]. Below T s , the spin-lattice relaxation rate from NMR experiments is enhanced as it captures the low-energy tail of the stripe spin-fluctuations [10,11]. Furthermore, recent µSR studies invoke the close proximity of FeSe to a magnetic quantum critical point as the muon relaxation rate shows unusual temperature dependence inside the nematic state [12].The changes in the electronic structure and magnetic fluctuations of FeSe can have profound implicatio...

The nematic electronic state and its associated nematic critical fluctuations have emerged as potential candidates for superconducting pairing in various unconventional superconductors. However, in most materials their coexistence with other magnetically-ordered phases poses significant challenges in establishing their importance. Here, by combining chemical and hydrostatic physical pressure in FeSe0.89S0.11, we provide a unique access to a clean nematic quantum phase transition in the absence of a long-range magnetic order. We find that in the proximity of the nematic phase transition, there is an unusual non-Fermi liquid behavior in resistivity at high temperatures that evolves into a Fermi liquid behaviour at the lowest temperatures. From quantum oscillations in high magnetic fields, we trace the evolution of the Fermi surface and electronic correlations as a function of applied pressure. We detect experimentally a Lifshitz transition that separates two distinct superconducting regions: one emerging from the nematic electronic phase with a small Fermi surface and strong electronic correlations and the other one with a large Fermi surface and weak correlations that promotes nesting and stabilization of a magnetically-ordered phase at high pressures. The lack of mass divergence suggests that the nematic critical fluctuations are quenched by the strong coupling to the lattice. This establishes that superconductivity is not enhanced at the nematic quantum phase transition in the absence of magnetic order.

We report theoretical and experimental evidence that EuCd2As2 in magnetic fields greater than 1.6 T applied along the c axis is a Weyl semimetal with a single pair of Weyl nodes. Ab initio electronic structure calculations, verified at zero field by angle-resolved photoemission spectra, predict Weyl nodes with wavevectors k = (0, 0, ±0.03) × 2π/c at the Fermi level when the Eu spins are fully aligned along the c axis. Shubnikov-de Haas oscillations measured in fields parallel to c reveal a cyclotron effective mass of m * c = 0.08 me and a Fermi surface of extremal area Aext = 0.24 nm −2 , corresponding to 0.1% of the area of the Brillouin zone. The small values of m * c and Aext are consistent with quasiparticles near a Weyl node. The identification of EuCd2As2 as a model Weyl semimetal opens the door to fundamental tests of Weyl physics.