Access and use of this website and the material on it are subject to the Terms and Conditions set forth at Inkjet printed thin and uniform dielectrics for capacitors and organic thin film transistors enabled by the coffee ring effect Graddage, Neil; Chu, Ta-Ya; Ding, Heping; Py, Christophe; Dadvand, Afshin; Tao, Ye http://nparc.cisti-icist.nrc-cnrc.gc.ca/npsi/jsp/nparc_cp.jsp?lang=fr L'accès à ce site Web et l'utilisation de son contenu sont assujettis aux conditions présentées dans le site LISEZ CES CONDITIONS ATTENTIVEMENT AVANT D'UTILISER CE SITE WEB.
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Biosensing
applications are driving an increase in demand for low-cost
photodetectors with sensitivity between 1000 and 1400 nm. Recently,
the sensitivity of Ag2Se colloidal quantum dot based devices
in this wavelength range has been observed. In this work we make the
first demonstration of an Ag2Se photodiode device with
sensitivity in this entire range. By employing secondary phosphine
to elevate the precursor reactivity, we achieved accurate size control
of the Ag2Se nanocrystals with a distinct excitonic absorption
peak. These nanocrystals were deposited from solution into a mesoporous
TiO2 scaffold, similar to that used in dye-sensitized solar
cells, to increase the light absorption and charge separation and
reduce the exciton diffusion length. By incorporation of a suitable
hole-transporting layer between the active layer and Ag anode, the
resulting devices showed a responsivity of 4.17 mA/W at a wavelength
of 1200 nm. These results demonstrate that Ag2Se colloidal
quantum dots offer a low-toxicity route for low-cost fabrication of
near-infrared photodetectors.
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