We study the transport properties of nonautonomous chaotic dynamical systems over a finite time duration. We are particularly interested in those regions that remain coherent and relatively non-dispersive over finite periods of time, despite the chaotic nature of the system. We develop a novel probabilistic methodology based upon transfer operators that automatically detects maximally coherent sets. The approach is very simple to implement, requiring only singular vector computations of a matrix of transitions induced by the dynamics. We illustrate our new methodology on an idealized stratospheric flow and in two and three dimensional analyses of European Centre for Medium Range Weather Forecasting (ECMWF) reanalysis data.

We describe a mathematical formalism and numerical algorithms for identifying and tracking slowly mixing objects in nonautonomous dynamical systems. In the autonomous setting, such objects are variously known as almost-invariant sets, metastable sets, persistent patterns, or strange eigenmodes, and have proved to be important in a variety of applications. In this current work, we explain how to extend existing autonomous approaches to the nonautonomous setting. We call the new time-dependent slowly mixing objects coherent sets as they represent regions of phase space that disperse very slowly and remain coherent. The new methods are illustrated via detailed examples in both discrete and continuous time.

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The "edge" of the Antarctic polar vortex is known to behave as a barrier to the meridional (poleward) transport of ozone during the austral winter. This chemical isolation of the polar vortex from the middle and low latitudes produces an ozone minimum in the vortex region, intensifying the ozone hole relative to that which would be produced by photochemical processes alone. Observational determination of the vortex edge remains an active field of research. In this letter, we obtain objective estimates of the structure of the polar vortex by introducing a new technique based on transfer operators that aims to find regions with minimal external transport. Applying this new technique to European Centre for Medium-Range Weather Forecasts (ECMWF) ERA-40 three-dimensional velocity data we produce an improved three-dimensional estimate of the vortex location in the upper stratosphere where the vortex is most pronounced. This novel computational approach has wide potential application in detecting and analysing mixing structures in a variety of atmospheric, oceanographic, and general fluid dynamical settings.