Abstract. We describe the construction of a continuous 38-year record of stratospheric aerosol optical properties. The Global Space-based Stratospheric Aerosol Climatology, or GloSSAC, provided the input data to the construction of the Climate Model Intercomparison Project stratospheric aerosol forcing data set and we have extended it through 2016 following an identical process. GloSSAC focuses on the Stratospheric Aerosol and Gas Experiment (SAGE) series of instruments through mid-2005, and on the Optical Spectrograph and InfraRed Imager System (OSIRIS) and the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) data thereafter. We also use data from other space instruments and from ground-based, air, and balloon borne instruments to fill in key gaps in the data set. The end result is a global and gap-free data set focused on aerosol extinction coefficient at 525 and 1020 nm and other parameters on an "as available" basis. For the primary data sets, we developed a new method for filling the post-Pinatubo eruption data gap for 1991-1993 based on data from the Cryogenic Limb Array Etalon Spectrometer. In addition, we developed a new method for populating wintertime high latitudes during the SAGE period employing a latitude-equivalent latitude conversion process that greatly improves the depiction of aerosol at high latitudes compared to earlier similar efforts. We report data in the troposphere only when and where it is available. This is primarily during the SAGE II period except for the most enhanced part of the Pinatubo period. It is likely that the upper troposphere during Pinatubo was greatly enhanced over non-volcanic periods and that domain remains substantially under-characterized. We note that aerosol levels during the OSIRIS/CALIPSO period in the lower stratosphere at mid-and high latitudes is routinely higher than what we observed during the SAGE II period. While this period had nearly continuous low-level volcanic activity, it is possible that the enhancement in part reflects deficiencies in the data set. We also expended substantial effort to quality assess the data set and the product is by far the best we have produced. GloSSAC version 1.0 is available in netCDF format at the NASA Atmospheric Data Center at https://eosweb.larc.nasa.gov/. GloSSAC users should cite this paper and the data set DOI (https://doi.org/10.5067/GloSSAC-L3-V1.0).

Aura Microwave Limb Sounder (MLS) measurements show that chemical processing was critical to the observed record‐low Arctic stratospheric ozone in spring 2020. The 16‐year MLS record indicates more polar denitrification and dehydration in 2019/2020 than in any Arctic winter except 2015/2016. Chlorine activation and ozone depletion began earlier than in any previously observed winter, with evidence of chemical ozone loss starting in November. Active chlorine then persisted as late into spring as it did in 2011. Empirical estimates suggest maximum chemical ozone losses near 2.8 ppmv by late March in both 2011 and 2020. However, peak chlorine activation, and thus peak ozone loss, occurred at lower altitudes in 2020 than in 2011, leading to the lowest Arctic ozone values ever observed at potential temperature levels from ∼400–480 K, with similar ozone values to those in 2011 at higher levels.

not only injected ash into the stratosphere but also large amounts of water vapor, breaking all records for direct injection of water vapor, by a volcano or otherwise, in the satellite era. This is not surprising since the Hunga Tonga-Hunga Ha'apai caldera was formerly situated 150 m below sea level. The massive blast injected water vapor up to altitudes as high as 53 km. Using measurements from the Microwave Limb Sounder on NASA's Aura satellite, we estimate that the excess water vapor is equivalent to around 10% of the amount of water vapor typically residing in the stratosphere. Unlike previous strong eruptions, this event may not cool the surface, but rather it could potentially warm the surface due to the excess water vapor. MILLÁN ET AL.

Aura Microwave Limb Sounder (MLS) measurements show that chemical processing was critical to the observed record-low Arctic stratospheric ozone in spring 2020. The 16-year MLS record indicates more polar denitrification and dehydration in 2019/2020 than in any Arctic winter except 2015/2016. Chlorine activation and ozone depletion began earlier than in any previously observed winter, with evidence of chemical ozone loss starting in November. Active chlorine then persisted as late into spring as it did in 2011. Empirical estimates suggest maximum chemical ozone losses near 2.8 ppmv by late March in both 2011 and 2020. However, peak chlorine activation, and thus peak ozone loss, occurred at lower altitudes in 2020 than in 2011, leading to the lowest Arctic ozone values ever observed at potential temperature levels from ∼400-480 K, with similar ozone values to those in 2011 at higher levels.Plain Language Summary Unlike the Antarctic, the Arctic does not usually experience an ozone hole because temperatures are often too high for the chemistry that destroys ozone. In 2019/2020, satellite measurements show record-low stratospheric wintertime temperatures and record-low springtime ozone concentrations in the Arctic lower stratosphere (about 12-to 20-km altitude). Only one other winter/spring season, 2010/2011, in this 16-year satellite data record comes close. Low temperatures, which result in chlorine being converted from nonreactive forms into forms that destroy ozone, started earlier than in any previous Arctic winter in the record and lingered later than in any year except 2011. The ozone-destroying chemistry in 2019/2020 occurred at lower altitudes (where more of the ozone that filters out harmful ultraviolet radiation resides) than in 2010/2011. Such extensive ozone loss can have important health and biological impacts because it leads to more ultraviolet radiation reaching the Earths surface. While the success of the Montreal Protocol in limiting human emissions that increase ozone-destroying gases in the stratosphere has resulted in much less Arctic ozone destruction than we would have otherwise had, future temperature changes could lead to other winters with even more chemical ozone depletion than in 2019/2020.

We describe the construction of a continuous 38-year record of stratospheric aerosol optical properties. The Global Space-based Stratospheric Aerosol Climatology, or GloSSAC, provided the input data to the 15 construction of the Climate Model Intercomparison Project stratospheric aerosol forcing data set (1979 to 2014) and we have extended it through 2016 following an identical process. GloSSAC focuses on the Stratospheric Aerosol and Gas Experiment (SAGE) series of instruments through mid-2005 and on the Optical Spectrograph and InfraRed Imager System (OSIRIS) and the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) data thereafter. We also use data from other space 20 instruments and from ground-based, air and balloon borne instruments to fill in key gaps in the data set. The end result is a global and gap-free data set focused on aerosol extinction coefficient at 525 and 1020 nm and other parameters on an 'as available' basis. For the primary data sets, we developed a new method for filling the post-Pinatubo eruption data gap for 1991 to 1993 based on data from the Cryogenic Limb Array Etalon Spectrometer. In addition, we developed a new method for populating wintertime high 25 latitudes during the SAGE period employing a latitude-equivalent latitude conversion process that greatly improves the depiction of aerosol at high latitudes compared to earlier similar efforts. We report data in the troposphere only when and where it is available. This is primarily during the SAGE II period except the most enhanced part of the Pinatubo period. It is likely that the upper troposphere during Pinatubo was greatly enhanced over non-volcanic periods and that domain remains substantially under characterized. 30We note that aerosol levels during the OSIRIS/CALIPSO period in the lower stratosphere at mid and high latitudes is routinely higher than what we observed during the SAGE II period. While this period had nearly continuous low-level volcanic activity, it is possible that the enhancement in part reflects deficiencies in the data set. We also expended substantial effort to quality assess the data set and the product is by far the best we have produced. GloSSAC version 1.0 is available in netCDF format at the NASA Atmospheric 35 Data Center at https://eosweb.larc.nasa.gov/. GloSSAC users should cite this paper and the data set DOI