Continuously tunable and coherent radiation in the wide range 56.8-1618 mum (0.18-5.27 THz) has been achieved as a novel and promising terahertz source based on collinear phase-matched difference frequency generation in a GaSe crystal. This source has the advantages of high coherence, simplicity for tuning, simple alignment, and stable output. The peak output power for the terahertz radiation reaches 69.4 W at a wavelength of 196 mum (1.53 THz), which corresponds to a photon conversion efficiency of 3.3%. A simple optimization of the design can yield a compact terahertz source.

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We report the extension of broadband degenerate OPO operation further into mid-infrared. A femtosecond thulium fiber laser with output centered at 2050 nm synchronously pumps a 500-μm-long crystal of orientation patterned GaAs providing broadband gain centered at 4.1 µm. We observe a pump threshold of 17 mW and output bandwidth extending from 2.6 to 6.1 µm at the -30 dB level. Average output power was 37 mW. Appropriate resonator group dispersion is a key factor for achieving degenerate operation with instantaneously broad bandwidth. The output spectrum is very sensitive to absorption and dispersion introduced by molecular species inside the OPO cavity.

Abstract:We present a new technique suitable for generating broadband phase-and frequency-locked frequency combs in the mid-infrared. Our source is based on a degenerate optical parametric oscillator (OPO) which rigorously both down-converts and augments the spectrum of a pump frequency comb provided by a commercial mode-locked near-IR laser. Low intracavity dispersion, combined with extensive cross-mixing of comb components, results in extremely broad instantaneous mid-IR bandwidths. We achieve an output power of 60 mW and 20dB bandwidth extending from 2500 to 3800 nm. Among other applications, such a source is wellsuited for coherent Fourier-transform spectroscopy in the absorption-rich mid-IR "molecular fingerprint" region.

We study coherence properties of a χ(²) optical parametric oscillator (OPO), which produces 2/3-octave-wide spectrum centered at the subharmonic (3120 nm) of the femtosecond pump laser. Our method consists of interfering the outputs of two identical, but independent OPOs pumped by the same laser. We demonstrate that the two OPOs show stable spatial and temporal interference and are mutually locked in frequency and in phase. By observing a collective heterodyne beat signal between the two OPOs we show that one can deterministically choose, by cavity length adjustment, between the two frequency states corresponding to the two sets of modes shifted with respect to each other by half of the laser pulse repetition rate. Moreover, we observe that the existence of two opposite phase states, a known common feature of a parametrically driven n = 2 subharmonic oscillator, reveals itself in our experiment as a common phase, 0 or π, being established through the whole set of some 300 thousand longitudinal modes.