We have compared the magnetic, transport, galvanomagnetic and specific heat properties of CeNiC2, PrNiC2 and NdNiC2 to study the interplay between charge density waves and magnetism in these compounds. The negative magnetoresistance in NdNiC2 is discussed in terms of the partial destruction of charge density waves and an irreversible phase transition stabilized by the field induced ferromagnetic transformation is reported. For PrNiC2 we demonstrate that the magnetic field initially weakens the CDW state, due to the Zeeman splitting of conduction bands. However, the Fermi surface nesting is enhanced at a temperature related to the magnetic anomaly.
Physical properties for the late lanthanide based RNiC2 (R = Dy, Ho, Er and Tm) ternary compounds are reported. All the compounds show antiferromagnetic ground state with the Néel temperature ranging from 3.4 K for HoNiC2 to 8.5 K for ErNiC2. The results of the transport and galvanomagnetic properties confirm a charge density wave state at and above room temperature with transition temperatures TCDW = 284 K, 335 K, 366 K, 394 K for DyNiC2, HoNiC2, ErNiC2 and TmNiC2, respectively. The Peierls temperature TCDW scales linearly with the unit cell volume. A similar linear dependence has been observed for the temperature of the lock-in transition T1 as well. Beyond the intersection point of the trend lines, the lock-in transition is no longer observed. In this article we demonstrate an extended phase diagram for RNiC2 family.
We report the specific heat, magnetic, magnetotransport and galvanomagnetic properties of polycrystalline GdNiC2. In the intermediate temperature region above TN = 20 K, we observe large negative magnetoresistance due to Zeeman splitting of the electronic bands and partial destruction of a charge density wave ground state. Our magnetoresistance and Hall measurements show that at low temperatures a magnetic field induced transformation from antiferromagnetic order to a metamagnetic phase results in the partial suppression of the CDW.
Detailed structural and magnetotransport properties of the monophosphate tungsten bronze Kx(PO2)4(WO3)8 single crystals are reported. Both galvanomagnetic and thermal properties are shown to be consistent with a charge density wave electronic transition due to hidden nesting of quasi -1D portion of the Fermi surface. We also observe the enhancement of electronic anisotropy due to reconstruction of the Fermi surface at the Peierls transition. The resistivity presents a thermal hysteresis suggesting a first order nature characteristics of a strong coupling scenario. However, other measurements such as the change of carriers density demonstrate a second order Peierls scenario with weak coupling features. We suggest that the structural transition driven by the residual strain in the K -P -O environment is responsible for the resistivity hysteresis and modifies the Fermi surface which then helps the rise to the second order Peierls instability.
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