Understanding the behavior of an impurity strongly interacting with a Fermi sea is a long-standing challenge in many-body physics. When the interactions are short ranged, two vastly different ground states exist: a polaron quasiparticle and a molecule dressed by the majority atoms. In the single-impurity limit, it is predicted that at a critical interaction strength, a first-order transition occurs between these two states. Experiments, however, are always conducted in the finite temperature and impurity density regime. The fate of the polaron-to-molecule transition under these conditions, where the statistics of quantum impurities and thermal effects become relevant, is still unknown. Here, we address this question experimentally and theoretically. Our experiments are performed with a spin-imbalanced ultracold Fermi gas with tunable interactions. Utilizing a novel Raman spectroscopy combined with a high-sensitivity fluorescence detection technique, we isolate the quasiparticle contribution and extract the polaron energy, spectral weight, and the contact parameter. As the interaction strength is increased, we observe a continuous variation of all observables, in particular a smooth reduction of the quasiparticle weight as it goes to zero beyond the transition point. Our observation is in good agreement with a theoretical model where polaron and molecule quasiparticle states are thermally occupied according to their quantum statistics. At the experimental conditions, polaron states are hence populated even at interactions where the molecule is the ground state and vice versa. The emerging physical picture is thus that of a smooth transition between polarons and molecules and a coexistence of both in the region around the expected transition. Our findings establish Raman spectroscopy as a powerful experimental tool for probing the physics of mobile quantum impurities and shed new light on the competition between emerging fermionic and bosonic quasiparticles in non-Fermi-liquid phases.

Shortcuts to adiabaticity are techniques allowing rapid variation of the system Hamiltonian without inducing excess heating. Fast optical transfer of atoms between different locations is an important application of shortcuts to adiabaticity. We show that the common boundary conditions on the atomic position, which are imposed to find the driving trajectory, lead to highly non-practical boundary conditions for the optical trap. Our experimental results demonstrate that, as a result, previously suggested trajectories are likely to fall short of the expectation. We develop two complementary methods that solve this boundary conditions problem by adding more degrees of freedom to the trajectory parameter space. In the first method, this is achieved by the addition of a spectral component at the trapping frequency, while in the second we use a polynomial trajectory of an order high enough to account for the new boundary conditions. We experimentally demonstrate that this approach allows us to construct highly non-adiabatic movements with no residual sloshing. Our techniques can also account for non-harmonic terms in the confining potential.

rf spectroscopy is one of the most powerful probing techniques in the field of ultracold gases. We report on a novel rf spectroscopy scheme with which we can detect very weak signals of only a few atoms. Using this method, we extended the experimentally accessible photon-energies range by an order of magnitude compared to previous studies. We directly verify a universal property of fermions with short-range interactions which is a power-law scaling of the rf spectrum tail all the way up to the interaction scale. We also determine, with high precision, the trap average contact parameter for different interaction strength. Finally, we employ our technique to precisely measure the binding energy of Feshbach molecules in an extended range of magnetic fields. These data are used to extract a new calibration of the Feshbach resonance between the two lowest energy levels of ^{40}K.

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