Organic materials exhibit exceptional room temperature light emitting characteristics and enormous exciton oscillator strength, however, their low charge carrier mobility prevent their use in high-performance applications such as electrically pumped lasers. In this context, ultralow threshold polariton lasers, whose operation relies on Bose-Einstein condensation of polaritons – part-light part-matter quasiparticles, are highly advantageous since the requirement for high carrier injection no longer holds. Polariton lasers have been successfully implemented using inorganic materials owing to their excellent electrical properties, however, in most cases their relatively small exciton binding energies limit their operation temperature. It has been suggested that combining organic and inorganic semiconductors in a hybrid microcavity, exploiting resonant interactions between these materials would permit to dramatically enhance optical nonlinearities and operation temperature. Here, we obtain cavity mediated hybridization of GaAs and J-aggregate excitons in the strong coupling regime under electrical injection of carriers as well as polariton lasing up to 200 K under non-resonant optical pumping. Our demonstration paves the way towards realization of hybrid organic-inorganic microcavities which utilise the organic component for sustaining high temperature polariton condensation and efficient electrical injection through inorganic structure.
We experimentally investigate the feasibility of a bolometric device based on exciton-polaritons. Initial measurements presented in this work show that heating – via thermal expansion and bandgap renormalization – modifies the exciton-polariton propagation wavevector making exciton-polaritons propagation remarkably sensitive to thermal variations. By theoretical simulations we predict that using a single layer graphene absorbing layer, a THz bolometric sensor can be realized by a simple exciton-polariton ring interferometer device. The predicted sensitivity is comparable to presently existing THz bolometric devices with the convenience of being a device that inherently produces an optical signal output.
Spatially confined, trapped polariton condensates have been shown to exhibit strong stochastic on-site spin polarization and in longer polariton condensate chains, distance controlled ferromagnetic and antiferromagnetic spin couplings. Until now, little is known, on how such polariton condensates spatially separated from their exciton reservoirs are trapped and formed. Here, we investigate the properties and formation dynamics of two main families of polariton condensates, those overlapping with the pump reservoir and those in confined geometries, under pulsed nonresonant excitation. The observed reduction in polariton condensation threshold and energy blueshift in trapped case is attributed to exciton reservoir-condensate spatial separation, whereas time-resolved photoluminescence measurements, reveal distinct relaxation and condensate formation dynamics with pair parametric scattering process being the dominant relaxation mechanism in trapped geometry.
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