We present the results of experimental and theoretical studies of high-order harmonic generation (HHG) in plasmas containing fullerenes using pulses of different duration and wavelength. We find that the harmonic cutoff is extended in the case of few-cycle pulses (3.5 fs, 29th harmonic) compared to longer laser pulses (40 fs, 25th harmonic) at the same intensity. Our studies also include HHG in fullerenes using 1300 and 780 nm multicycle (35 and 40 fs) pulses. For 1300 nm pulses, an extension of the harmonic cutoff to the 41st order was obtained, with a decrease in conversion efficiency that is consistent with theoretical predictions based on wave packet spreading for single atoms. Theoretical calculations of fullerene harmonic spectra using the single active electron approximation were carried out for both few-cycle and multicycle pulses.
The tunneling ionization of exotic atoms such as muonic hydrogen, muonium and positronium in a strong laser field of circular polarization is investigated taking into account the impact of the motion of the center of mass on the the tunneling ionization dynamics. The momentum partition between the ionization products is deduced. The effect of the center of mass motion for the momentum distribution of the ionization components is determined. The effect scales with the ratio of the electron (muon) to the atomic core masses and is nonnegligible for exotic atoms, while being insignificant for common atoms. It is shown that the electron (muon) momentum shift during the under-the-barrier motion due to the magnetically induced Lorentz force has a significant impact on the momentum distribution of the atomic core and depends on the ratio of the electron to the atomic core masses
The time-dependent wave function of a nanoring driven by a laser field is obtained by exploiting the symmetries\ud
inherent to the system and used for studying the properties of the electromagnetic radiation emitted by the\ud
nanoring as a function of the polarization state of the laser. The diffused radiation has the characteristics of\ud
high-order-harmonic generation. For a noncircularly polarized laser field an extension of the expected cutoff\ud
position is evident, indicating that nanorings are efficient sources of radiation. The polarization state of the\ud
emitted harmonics can be opportunely controlled by varying the parameters of the pump field. The profile of\ud
the absorbed angular moment shows that a magnetic moment can be induced depending on the polarization of\ud
the driven field
We discuss the physical properties of a noninteracting electron gas constrained to a spherical surface. In particular we consider its chemical potentials, its ionization potential, and its electric static polarizability. All these properties are discussed analytically as functions of the number N of electrons. The trends obtained with increasing N are compared with those of the corresponding properties experimentally measured or theoretically evaluated for quasispherical hollow atomic and molecular clusters. Most of the properties investigated display similar trends, characterized by a prominence of shell effects. This leads to the definition of a scale-invariant distribution of magic numbers which follows a power law with critical exponent −0.5. We conclude that our completely mechanistic and analytically tractable model can be useful for the analysis of self-assembling complex systems.
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