The final stable shape taken by a fluid–fluid interface when it experiences a growing instability can be important in determining features as diverse as weather patterns in the atmosphere and oceans, the growth of cell structures and viruses, and the dynamics of planets and stars. An example which is accessible to laboratory study is that of an air bubble driven by ultrasound when it becomes shape-unstable through a parametric instability. Above the critical driving pressure threshold for shape oscillations, which is minimal at the resonance of the breathing mode, regular patterns of surface waves are observed on the bubble wall. The existing theoretical models, which take account only of the interaction between the breathing and distortion modes, cannot explain the selection of the regular pattern on the bubble wall. This paper proposes an explanation which is based on the consideration of a three-wave resonant interaction between the distortion modes. Using a Hamiltonian approach to nonlinear bubble oscillation, corrections to the dynamical equations governing the evolution of the amplitudes of interacting surface modes have been derived. Steady-state solutions of these equations describe the formation of a regular structure. Our predictions are confirmed by images of patterns observed on the bubble wall.
This paper reports on noninertial cavitation that occurs beyond the zone close to the horn tip to which the inertial cavitation is confined. The noninertial cavitation is characterized by collating the data from a range of measurements of bubbles trapped on a solid surface in this noninertial zone. Specifically, the electrochemical measurement of mass transfer to an electrode is compared with high-speed video of the bubble oscillation. This gas bubble is shown to be a "noninertial" event by electrochemical surface erosion measurements and "ring-down" experiments showing the activity and motion of the bubble as the sound excitation was terminated. These measurements enable characterization of the complex environment produced below an operating ultrasonic horn outside of the region where inertial collapse can be detected. The extent to which solid boundaries in the liquid cause the frequencies and shapes of oscillatory modes on the bubble wall to differ from their free field values is discussed.
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