We report the coexistence of ferromagnetic order and superconductivity in UCoGe at ambient pressure. Magnetization measurements show that UCoGe is a weak ferromagnet with a Curie temperature T C 3 K and a small ordered moment m 0 0:03 B . Superconductivity is observed with a resistive transition temperature T s 0:8 K for the best sample. Thermal-expansion and specific-heat measurements provide solid evidence for bulk magnetism and superconductivity. The proximity to a ferromagnetic instability, the defect sensitivity of T s , and the absence of Pauli limiting, suggest triplet superconductivity mediated by critical ferromagnetic fluctuations. DOI: 10.1103/PhysRevLett.99.067006 PACS numbers: 74.70.Tx, 74.20.Mn, 75.30.Kz In the standard theory for superconductivity (SC) due to Bardeen, Schrieffer, and Cooper ferromagnetic (FM) order impedes the pairing of electrons in singlet states [1]. It has been argued, however, that on the border line of ferromagnetism, critical magnetic fluctuations could mediate SC by pairing the electrons in triplet states [2]. The discovery several years ago of SC in the metallic ferromagnets UGe 2 (at high pressure) [3], URhGe [4], and possibly UIr (at high pressure) [5], has put this idea on firm footing. However, later work provided evidence for a more intricate scenario in which SC in UGe 2 and URhGe is driven by a magnetic transition between two polarized phases [6 -8] rather than by critical fluctuations associated with the zero temperature transition from a paramagnetic to a FM phase. Here we report a novel ambient-pressure FM superconductor UCoGe. Since SC occurs right on the border line of FM order, UCoGe may present the first example of SC stimulated by critical fluctuations associated with a FM quantum critical point (QCP).UCoGe belongs to the family of intermetallic UTX compounds, with T a transition metal and X is Si or Ge, that was first manufactured by Troć and Tran [9]. UCoGe crystallizes in the orthorhombic TiNiSi structure (space group P nma ) [10,11], just like URhGe. From magnetization, resistivity (T 4:2 K) [9,10] and specific-heat measurements (T 1:2 K) [12] it was concluded that UCoGe has a paramagnetic ground state. This provided the motivation to alloy URhGe (Curie temperature T C 9:5 K) with Co in a search for a FM QCP in the series URh 1ÿx Co x Ge (x 0:9) [13]. Magnetization data showed that T C upon doping first increases, has a broad maximum near x 0:6 (T max C 20 K) and then rapidly drops to 8 K for x 0:9 [13]. This hinted at a FM QCP for x & 1:0. In this Letter we show that the end (x 1:0) compound UCoGe is in fact a weak itinerant ferromagnet. Moreover, metallic ferromagnetism coexists with SC below 0.8 K at ambient pressure.Polycrystalline UCoGe samples were prepared with nominal compositions U 1:02 CoGe (sample 2) and U 1:02 Co 1:02 Ge (sample 3) by arc melting the constituents (natural U 99.9%, Co 99.9%, and Ge 99.999%) under a high-purity argon atmosphere in a water-cooled copper crucible. The as-cast samples were annealed for 10 days at 850 C. Sampl...
By muon spin-relaxation measurements on single-crystal specimens, we show that superconductivity in the AFe 2 As 2 ͑A =Ca,Ba,Sr͒ systems, in both the cases of composition and pressure tunings, coexists with a strong static magnetic order in a partial volume fraction. The superfluid response from the remaining paramagnetic volume fraction of ͑Ba 0.5 K 0.5 ͒Fe 2 As 2 exhibits a nearly linear variation in T at low temperatures, suggesting an anisotropic energy gap with line nodes and/or multigap effects.
Chiral nematic liquid crystals sometimes form blue phases characterized by spirals twisting in different directions. By combining model calculations with neutron-scattering experiments, we show that the magnetic analogue of blue phases does form in the chiral itinerant magnet MnSi in a large part of the phase diagram. The properties of this blue phase explain a number of previously reported puzzling features of MnSi such as partial magnetic order and a two-component specific-heat and thermal-expansion anomaly at the magnetic transition.
In superconducting copper oxides some Cu-O bond-stretching phonons around 70meV show anomalous giant softening and broadening of electronic origin and electronic dispersions have large renormalization kinks near the same energy. These observations suggest that phonon broadening originates from quasiparticle excitations across the Fermi surface and the electronic dispersion kinks originate from coupling to anomalous phonons. We measured the phonon anomaly in underdoped (x=0.05) and overdoped (x=0.20,0.25) La2−xSrxCuO4 by inelastic neutron and x-ray scattering with high resolution. Combining these and previously published data, we found that doping-dependence of the magnitude of the giant phonon anomaly is very different from that of the ARPES kink, i.e. the two phenomena are not connected. We show that these results provide indirect evidence that the phonon anomaly originates from novel collective charge excitations as opposed to interactions with electron-hole pairs. Their amplitude follows the superconducting dome so these charge modes may be important for superconductivity.PACS numbers: 74.25.Kc, 63.20.kd, 74.20.Mn Lattice vibrations in metals can be damped and/or softened by either electronic quasiparticles or collective charge excitations (e.g. plasmons). Giant phonon softening and line broadening of electronic origin of the longitudinal Cu-O bond stretching phonons near half-way to the zone boundary (giant anomaly) was observed in copper oxide high temperature superconductors (HTSCs) 1-11 . It was previously found at superconducting compositions and was also absent in undoped and overdoped nonsuperconducting copper oxides [5][6][7] .First reports interpreted the phonon anomaly as a signature of unit cell doubling 3 followed by a different interpretation 6 in terms of coupling of the phonon to dynamic charge stripes. Subsequently, close kinematic relationship between the longitudinal Cu-O bond stretching mode dispersion and renormalization of electronic quasiparticles in Bi 2 Sr 1.6 La 0.4 CuO 6 (Bi2201) indicated that the phonon anomaly may originate from the coupling of phonons to electronic quasiparticles 11 . t − J modelbased calculations also predicted strong coupling of optical phonons to electron-hole excitations 12 .If phonons couple strongly to electronic quasipaticles, then a BCS-type mechanism of superconductivity may still be valid. Alternatively, the phonon anomaly would arise from a novel collective charge excitations at low energies (at least 70 meV). Then such collective mode may provide the pairing interaction 13-15 .We measured Cu-O bond-stretching phonons in La 2−x Sr x CuO 4 for undoped x=0.00, nonsuperconducting underdoped x=0.05, and superconducting overdoped x=0.20, 0.25. x=0.05 did not show characteristic signatures of the giant phonon anomaly. x=0.20 showed a very strong phonon anomaly, which was dramatically reduced already at x=0.25. On the other hand, the magnitude of the kink in the electronic dispersions gradually decreases from x=0.05 to x=0.30 16,17 . The new data, combine...
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