A high-energy supercontinuum spanning 4.7 octaves, from 250 to 6500 nm, is generated using a 0.3-TW, 3.9-μm output of a mid-infrared optical parametric chirped-pulse amplifier as a driver inducing a laser filament in the air. The high-frequency wing of the supercontinuum spectrum is enhanced by odd-order optical harmonics of the mid-infrared driver. Optical harmonics up to the 15th order are observed in supercontinuum spectra as overlapping, yet well-resolved peaks broadened, as verified by numerical modeling, due to spatially nonuniform ionization-induced blue shift.
Optical breathing solitons are known to display well-resolved cycles where the phase of pulse compression is followed by pulse stretching. Here we show that, in the extreme regimes where the soliton pulse width approaches the field cycle, the field waveform dynamics can drastically differ from this textbook scenario. We demonstrate that such extremely short soliton transients can develop optical shock waves, which seed parametric amplification, facilitating, along with ionization nonlinearity, soliton compression to subcycle pulse widths. This pulse compression scenario is shown to enable the generation of sub-quarter-cycle multigigawatt optical field waveforms in the mid infrared.
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